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If Librarian boost himself with the spell, can he:
- run than shoot or
- run twice or
- shoot than heal
in one attack phase.
No. The quickening specifically states he can attack twice with his bolt pistol and sword - it doesn't give him the option to do anything else. Even if it did effectively give him two "actions", combat recovery and running are actions that are done "instead of attacking" (in other words, you don't get to make any attacks that round, even if you are entitle to make several).